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Surface underway data from the R/V Marcus G. Langseth spans the Arctic Ocean, Beaufort Sea, Bering Sea, Caribbean Sea, and multiple U.S. National Marine Sanctuaries from 2010-05-07 to 2013-06-25. The dataset includes measurements of the partial pressure (or fugacity) of carbon dioxide in water, salinity, and sea surface temperature. It was collected by researchers from Columbia University's Lamont-Doherty Earth Observatory and the University of Colorado using carbon dioxide gas analyzers and equilibrators.
Dataset appears on multiple platforms (NASA Earthdata, Data.gov) but with incomplete metadata. The primary format listed is HTML, which may not be the raw data format.